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It's from the sixth episode of the first season of Breaking Bad. The context is one guys took another guy to a drug distributor to sell him drugs. The guy hands him a pack of meth, but the drug dealer refuses to give him money.
Guy A: You said this was cool, okay! Money for meth, cash upfont.
Guy B: Don't front, dude! Tuco's good for it.
To front is slang meaning to make pretense, to cop an attitude, or to get too upset inappropriately.
In other words...
Don’t get upset. You know Tuco is good for it. He will pay you back. He is worthy of a little credit.
